GHz bandwidth electro-optics of a single self-assembled quantum dot in a charge-tunable device

The response of a single InGaAs quantum dot, embedded in a miniaturized charge-tunable device, to an applied GHz bandwidth electrical pulse is investigated via its optical response. Quantum dot response times of 1.0 \pm 0.1 ns are characterized via several different measurement techniques, demonstrating GHz bandwidth electrical control. Furthermore a novel optical detection technique based on resonant electron-hole pair generation in the hybridization region is used to map fully the voltage pulse experienced by the quantum dot, showing in this case a simple exponential rise.Comment: 7 pages, 4 figure

Ultracold collision properties of metastable alkaline-earth atoms

Ultra-cold collisions of spin-polarized 24Mg,40Ca, and 88Sr in the metastable 3P2 excited state are investigated. We calculate the long-range interaction potentials and estimate the scattering length and the collisional loss rate as a function of magnetic field. The estimates are based on molecular potentials between 3P2 alkaline-earth atoms obtained from ab initio atomic and molecular structure calculations. The scattering lengths show resonance behavior due to the appearance of a molecular bound state in a purely long-range interaction potential and are positive for magnetic fields below 50 mT. A loss-rate model shows that losses should be smallest near zero magnetic field and for fields slightly larger than the resonance field, where the scattering length is also positive.Comment: 4 pages, 4 figure

Nanometric depth resolution from multi-focal images in microscopy

We describe a method for tracking the position of small features in three dimensions from images recorded on a standard microscope with an inexpensive attachment between the microscope and the camera. The depth-measurement accuracy of this method is tested experimentally on a wide-field, inverted microscope and is shown to give approximately 8 nm depth resolution, over a specimen depth of approximately 6 µm, when using a 12-bit charge-coupled device (CCD) camera and very bright but unresolved particles. To assess low-flux limitations a theoretical model is used to derive an analytical expression for the minimum variance bound. The approximations used in the analytical treatment are tested using numerical simulations. It is concluded that approximately 14 nm depth resolution is achievable with flux levels available when tracking fluorescent sources in three dimensions in live-cell biology and that the method is suitable for three-dimensional photo-activated localization microscopy resolution. Sub-nanometre resolution could be achieved with photon-counting techniques at high flux levels

Near-Infrared Spectroscopy of Molecular Filaments in the Reflection Nebula NGC 7023

We present near-infrared spectroscopy of fluorescent molecular hydrogen (H_2) emission from molecular filaments in the reflection nebula NGC 7023. We derive the relative column densities of H_2 rotational-vibrational states from the measured line emission and compare these results with several model photodissociation regions covering a range of densities, incident UV-fields, and excitation mechanisms. Our best-fit models for one filament suggest, but do not require, either a combination of different densities, suggesting clumps of 10^6 cm^{-3} in a 10^4 - 10^5 cm^{-3} filament, or a combination of fluorescent excitation and thermally-excited gas, perhaps due to a shock from a bipolar outflow. We derive densities and UV fields for these molecular filaments that are in agreement with previous determinations.Comment: ApJ accepted, 26 pages including 5 embedded figures, uses AASTEX. Also available at http://www-astronomy.mps.ohio-state.edu/~martini/pubs.htm

Near-Infrared Spectroscopy of Molecular Hydrogen Emission in Four Reflection Nebulae: NGC 1333, NGC 2023, NGC 2068, and NGC 7023

We present near-infrared spectroscopy of fluorescent molecular hydrogen (H_2) emission from NGC 1333, NGC 2023, NGC 2068, and NGC 7023 and derive the physical properties of the molecular material in these reflection nebulae. Our observations of NGC 2023 and NGC 7023 and the physical parameters we derive for these nebulae are in good agreement with previous studies. Both NGC 1333 and NGC 2068 have no previously-published analysis of near-infrared spectra. Our study reveals that the rotational-vibrational states of molecular hydrogen in NGC 1333 are populated quite differently from NGC 2023 and NGC 7023. We determine that the relatively weak UV field illuminating NGC 1333 is the primary cause of the difference. Further, we find that the density of the emitting material in NGC 1333 is of much lower density, with n ~ 10^2 - 10^4 cm^-3. NGC 2068 has molecular hydrogen line ratios more similar to those of NGC 7023 and NGC 2023. Our model fits to this nebula show that the bright, H_2-emitting material may have a density as high as n ~ 10^5 cm^-3, similar to what we find for NGC 2023 and NGC 7023. Our spectra of NGC 2023 and NGC 7023 show significant changes in both the near-infrared continuum and H_2 intensity along the slit and offsets between the peaks of the H_2 and continuum emission. We find that these brightness changes may correspond to real changes in the density and temperatures of the emitting region, although uncertainties in the total column of emitting material along a given line of sight complicates the interpretation. The spatial difference in the peak of the H_2 and near-infrared continuum peaks in NGC 2023 and NGC 7023 shows that the near-infrared continuum is due to a material which can survive closer to the star than H_2 can.Comment: Submitted for publication in ApJ. 34 pages including 12 embedded postscript figures. Also available at http://www.astronomy.ohio-state.edu/~martini/pub

表紙・目次

The photophysical behavior of conjugated polymers used in modern optoelectronic devices is strongly influenced by their structural dynamics and conformational heterogeneity, both of which are dependent on solvent properties. Single molecule studies of these polymer systems embedded in a host matrix have proven to be very powerful to investigate the fundamental fluorescent properties. However, such studies lack the possibility of examining the relationship between conformational dynamics and photophysical response in solution, which is the phase from which films for devices are deposited. By developing a synthetic strategy to incorporate a biotin moiety as a surface attachment point at one end of a polyalkylthiophene, we immobilize it, enabling us to make the first single molecule fluorescence measurements of conjugated polymers for long periods of time in solution. We identify fluctuation patterns in the fluorescence signal that can be rationalized in terms of photobleaching and stochastic transitions to reversible dark states. Moreover, by using the advantages of solution-based imaging, we demonstrate that the addition of oxygen scavengers improves optical stability by significantly decreasing the photobleaching rates.<br/